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西藏城市大气臭氧质量浓度变化及其影响

陈熠 郭淑政 张田甜 林伟立

陈熠, 郭淑政, 张田甜, 等. 西藏城市大气臭氧质量浓度变化及其影响. 应用气象学报, 2024, 35(6): 715-724. DOI:  10.11898/1001-7313.20240607..
引用本文: 陈熠, 郭淑政, 张田甜, 等. 西藏城市大气臭氧质量浓度变化及其影响. 应用气象学报, 2024, 35(6): 715-724. DOI:  10.11898/1001-7313.20240607.
Chen Yi, Guo Shuzheng, Zhang Tiantian, et al. Variations of ozone concentration with its impacts on cities of Xizang. J Appl Meteor Sci, 2024, 35(6): 715-724. DOI:  10.11898/1001-7313.20240607.
Citation: Chen Yi, Guo Shuzheng, Zhang Tiantian, et al. Variations of ozone concentration with its impacts on cities of Xizang. J Appl Meteor Sci, 2024, 35(6): 715-724. DOI:  10.11898/1001-7313.20240607.

西藏城市大气臭氧质量浓度变化及其影响

DOI: 10.11898/1001-7313.20240607
资助项目: 

国家自然科学基金项目 21876214

详细信息
    通信作者:

    林伟立, 邮箱: linwl@muc.edu.cn

Variations of Ozone Concentration with Its Impacts on Cities of Xizang

  • 摘要: 在强紫外线辐射和高臭氧(O3)背景值下, 人为排放源集中的青藏高原城市地区大气O3质量浓度长期变化及其潜在环境影响备受关注。该研究收集2015—2023年西藏7个城市的O3质量浓度数据, 分析其变化趋势, 并借助13个O3风险评价指标评估O3对当地居民健康和生态植被的潜在威胁。结果表明:O3质量浓度在拉萨明显高于南部的山南和日喀则, 与北部的那曲相当, 高于西部的阿里以及东部的林芝和昌都。昌都O3峰值出现在6月, 林芝O3峰值出现在3—4月, 其他城市则出现在5月。阿里、那曲、拉萨和林芝的O3质量浓度呈年际波动, 山南、日喀则和昌都的O3质量浓度呈显著上升趋势。健康与生态O3风险指标与日间O3质量浓度紧密相关。相比西藏其他城市, 拉萨的O3暴露带来的影响尤为突出, 部分风险指标已突破安全阈值。在高O3背景值基础上, 由于人为排放的不断增加, 西藏城市须采取有效的O3预防和控制措施, 以长期维护青藏高原城市地区大气环境质量。
  • 图  1  西藏7个城市O3质量浓度平均年变化(a)与日变化(b)

    Fig. 1  Averaged annual variation(a) and diurnal variation(b) of O3 mass concentrations of 7 cities in Xizang

    图  2  西藏7个城市O3风险指标比较

    Fig. 2  Comparison of O3 exposure risk metric among 7 cities in Xizang

    图  3  西藏7个城市的SdAVG指数季节平均变化

    Fig. 3  Averaged seasonal variations in SdAVG of 7 cities in Xizang

    图  4  西藏7个城市AOT40的季节变化

    Fig. 4  Seasonal variations in AOT40 of 7 cities in Xizang

    图  5  西藏7个城市W126的季节变化

    Fig. 5  Seasonal variations in W126 of 7 cities in Xizang

    表  1  O3风险评价指标

    Table  1  Definition of O3 evaluation metrics

    指标名称 简称 单位 主要用途 文献来源
    所有小时O3质量浓度年平均值 AAVG μg·m-3 环境变化 [14]
    所有白天(10:00—21:59)小时O3质量浓度年平均值 AdAVG μg·m-3 环境变化 [14]
    不同季节所有小时O3质量浓度平均值 SAVG μg·m-3 环境变化 [14]
    不同季节白天(10:00—21:59)小时O3质量浓度平均值 SdAVG μg·m-3 环境变化 [14]
    日连续8 h平均O3质量浓度最大值 MDA8 μg·m-3 人体健康
    日连续8 h平均O3质量浓度年最大值 AMDA8_max μg·m-3 人体健康 [14]
    日连续8 h O3质量浓度年第4高值 AMDA8_4th μg·m-3 人体健康 [14]
    日连续8 h O3质量浓度最大值与69 μg·m-3正差值的年总和 SOMO35 μg·m-3·d 人体健康 [21]
    日连续8 h O3质量浓度最大值与69 μg·m-3之间的正差值的季节总和 SSOMO35 μg·m-3·d 人体健康 [21]
    每年MDA8大于176 μg·m-3的日数 NDGT90 d 人体健康 [14]
    每年MDA8大于137 μg·m-3的日数 NDGT70 d 人体健康 [14]
    3个月内所有白天(10:00—21:59)小时O3质量浓度与78 μg·m-3正差值总和 AOT40 μg·m-3·h 生态植被 [22]
    3个月内所有白天(10:00—21:59)小时O3浓度质量加权总和 W126 μg·m-3·h 生态植被 [23]
    下载: 导出CSV

    表  2  西藏7个城市的年平均O3质量浓度变化(单位:μg·m-3)

    Table  2  Variations in annual O3 mass concentrations of 7 cities in Xizang(unit:μg·m-3)

    年份 阿里 那曲 拉萨 山南 日喀则 林芝 昌都
    2015 63.3±29.2 64.8±31.7 80.1±33.1 75.2±27.4 52.3±27.8 68.0±28.8 58.4±25.1
    2016 67.4±36.4 75.4±28.6 77.2±38.6 78.2±36.6 33.3±22.3 62.1±28.4 42.9±18.0
    2017 64.5±33.9 84.4±33.3 73.9±31.5 73.7±31.7 46.0±21.4 69.0±29.0 89.7±31.7
    2018 64.7±32.1 85.8±31.9 80.7±32.5 82.1±31.7 53.7±24.3 75.2±30.0 79.9±32.1
    2019 57.2±28.4 78.8±26.8 75.8±29.8 79.3±32.5 56.6±24.3 67.6±25.3 78.6±30.2
    2020 60.0±25.9 74.6±26.3 72.1±28.8 80.1±29.8 61.5±24.7 65.0±25.9 89.9±32.7
    2021 66.4±27.6 74.3±25.5 73.9±27.0 80.5±29.6 72.9±31.0 62.1±25.1 96.4±30.8
    2022 68.6±26.6 83.9±27.0 82.3±26.1 84.6±29.2 77.0±29.2 68.4±24.1 98.2±29.8
    2023 67.8±29.0 80.5±26.8 87.2±33.1 82.7±31.2 80.3±27.8 71.9±28.0 92.5±29.2
    下载: 导出CSV

    表  3  西藏7个城市不同O3指标的年变化趋势

    Table  3  Annual trends in different O3 metrics of 7 cities in Xizang

    城市 AAVG/(μg·m-3·a-1) AdAVG/(μg·m-3·a-1) AMDA8_max/(μg·m-3·a-1) AMDA8_4th/(μg·m-3·a-1) SOMO35/(μg·m-3·a-1) NDGT90/(d·a-1) NDGT70/(d·a-1)
    阿里 0.18 -0.19 -6.50* -0.66 -120 -0* -2
    那曲 0.48 0.39 -1.34 -1.29 9 -0 -1
    拉萨 0.30 -0.02 -2.01* -1.32 -30 -1 -2
    山南 0.51* 0.50* -1.49 -0.12 121 -0 2
    日喀则 2.60* 2.76* 2.66 2.82* 613* -0 2*
    林芝 0.09 -0.08 -2.82 -0.87 -43 -0 -1
    昌都 2.76* 3.02* 3.53 3.56* 731* 1 7*
    注:* 表示达到0.05显著性水平。
    下载: 导出CSV

    表  4  西藏7个城市的不同季节O3指标的变化趋势

    Table  4  Trends of O3 metrics in different seasons of 7 cities in Xizang

    城市 季节 SAVG/(μg·m-3·a-1) SdAVG/(μg·m-3·a-1) SSOMO35/(μg·m-3·d·a-1) AOT40/(μg·m-3·h·a-1) W126/(μg·m-3·h·a-1)
    阿里 0.13 -0.25 -34 -216 -551
    -0.01 -0.37 -55 -261 -366
    0.28 -0.17 -29 -157 -87
    -0.06 -0.32 -45 -261 -178
    那曲 1.34 1.34 84 729 500
    -0.23 -0.36 -34 -279 -453
    -0.08 -0.31 -35 -218 -169
    -0.46 -0.57 -80 -484 -350
    拉萨 0.01 -0.38 -46 -133 -614
    0.07 -0.23 -26 -206 -366
    0.81 0.33 24 229 195
    -0.11 -0.12 -37 -189 -110
    山南 0.62 0.69 58 776 938
    0.64 0.67 44 411 519
    0.48 0.35 27 258* 169
    -0.35 -0.18 -50 -261 -228
    日喀则 2.33* 2.41* 211* 1832* 1849*
    3.00* 3.31* 208* 1639* 1686*
    2.75* 2.79* 145* 777 539*
    2.07* 2.11* 59 278 166
    林芝 0.16 -0.01 -6 80 -111
    -0.01 -0.26 -27 -194 -215
    -0.01 -0.18 -16 -112 -48
    -0.38 -0.41 -51 -280 -188
    昌都 2.56 2.75 207* 1931* 2370*
    3.87* 4.26* 338* 3015* 4169*
    2.55* 2.83* 172* 1168* 949
    1.75 2.06 68 399 255
    注:* 表示达到0.05显著性水平。
    下载: 导出CSV
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  • 收稿日期:  2024-07-04
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