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我国北方地区对流层中下层臭氧收支

彭丽 林云萍 周广强 赵春生 耿福海

彭丽, 林云萍, 周广强, 等. 我国北方地区对流层中下层臭氧收支. 应用气象学报, 2009, 20(6): 665-672..
引用本文: 彭丽, 林云萍, 周广强, 等. 我国北方地区对流层中下层臭氧收支. 应用气象学报, 2009, 20(6): 665-672.
Peng Li, Lin Yunping, Zhou Guangqiang, et al. Ozone budget in the lower and middle troposphere over North China. J Appl Meteor Sci, 2009, 20(6): 665-672.
Citation: Peng Li, Lin Yunping, Zhou Guangqiang, et al. Ozone budget in the lower and middle troposphere over North China. J Appl Meteor Sci, 2009, 20(6): 665-672.

我国北方地区对流层中下层臭氧收支

资助项目: 

国家自然科学基金项目 40575060

Ozone Budget in the Lower and Middle Troposphere over North China

  • 摘要: 为了揭示我国北方地区对流层中下层臭氧(O3) 的形成机理以及周边地区的污染输送对我国北方地区对流层中下层O3收支的影响, 在与外场观测数据比较分析的基础上, 利用全球化学输送模式(MOZART-2) 采用收支分析方法定量分析了影响我国北方地区对流层中下层O3的各个物理化学过程。结果表明:我国北方地区对流层下层O3最重要的来源是光化学生成作用, 约占总来源的58.3%(41.5 Tg), 光化学生成反应中HO2对于O3生成的贡献最大; 最大的汇是干沉降过程, 约占总汇的43.2%(26.2Tg); 水平净输送作用对我国北方地区对流层中下层O3收支的影响非常大, 在我国北方地区对流层下层, 41.6%左右的O3来自水平净输送, 随高度增加, 水平输送影响增大, 我国北方地区对流层中层大约81.5%的O3来自水平净输送。
  • 图  1  地面至25km的O3浓度模拟值与观测值比对

    Fig. 1  Comparison of simulated O3 with the observed from ground to 25 km

    图  2  地面至12km的O3浓度模拟值与观测值比对

    Fig. 2  Comparison of simulated O3 with the observed from ground to 12 km

    图  3  2004年我国北方地区臭氧光化学收支年变化

    (a) 对流层下层, (b) 对流层中层

    Fig. 3  Annual circle of O3 photochemical budget in North China of 2004

    (a) lower troposphere, (b) middle troposphere

    图  4  2004年我国北方地区的O3干沉降年变化

    Fig. 4  Annual circle of O3 dry deposition in North China of 2004

    图  5  2004年我国北方地区的O3水平输送量年变化

    (a) 对流层下层, (b) 对流层中层

    Fig. 5  Annual circle of O3 horizontal transport in North China of 2004

    (a) lower troposphere, (b) middle troposphere

    表  1  2004年我国北方地区对流层中下层O3年收支(单位:Tg)

    Table  1  Annual O3 budget in the lower and middle troposphere over North China of 2004 (unit:Tg)

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出版历程
  • 收稿日期:  2009-02-17
  • 修回日期:  2009-10-08
  • 刊出日期:  2009-12-31

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